Boosting hydrogen spillover with carbon modification: A path to high-performance Cu-ZnO-ZrO2 catalyst for CO2 hydrogenation to methanol
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Y Jin, X Sun, H Zhong, Z Cheng, G Lan, S Wei…
Applied Catalysis B …, 2025
Elsevier
The Cu-based catalysts for CO 2 hydrogenation to methanol still face challenges in achieving satisfactory methanol selectivity. Typically, the hydrogenation of intermediates is regarded as the rate-determining step, making the acceleration of hydrogenation dynamics a critical priority in developing highly efficient catalysts for methanol synthesis. Herein, we develop a carbon modified Cu-ZnO-ZrO 2 catalyst through an in-situ pyrolysis carbonization strategy with β-cyclodextrin (CD) as carbon source, where the carbon species are in intimate …
