Regulation of Interfacial Ion Transport via Honeycomb‐Architected Covalent Organic Frameworks for Lithium Metal Batteries
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Y Chen, J He, M Li, H Shen, C Han, Y Tian…
Advanced …, 2025
Wiley Online Library
This study pioneers vertically aligned honeycomb covalent organic framework (HCCOF) on graphene oxide (HCCOF‐GO) through one‐pot colloidal assembly, establishing a paradigm for interface‐engineered 2D heterostructures in lithium metal batteries (LMBs). Mechanistically, the vertical COF alignment via interfacial π–π conjugation preserves intrinsic 1.15 nm hexagonal pores while integrating Go's electron transport capabilities. When deployed as an artificial solid‐electrolyte interphase (ASEI), this architecture …
